O-M-403-15 The Effect of Synthesis Methods on the Evolution of Isolated Atom Catalysts during Propane Dehydrogenation

Monday, June 15, 2015: 4:40 PM
403-405 (Lawrence Convention Center)
Bo Hu1, Andrew Getsoian2, Guanghui Zhang1, Ujjal Das2, Jeffrey Camacho-Bunquin2, Peter C. Stair2,3, Christopher L. Marshall2, Jeffrey T. Miller2, Larry Curtiss2 and Adam S. Hock1,2, (1)Illinois Institute of Technology, USA, (2)Argonne National Laboratory, USA, (3)Northwestern University, USA.
This talk details a comparision of aqueous, organometallic, and ALD syntheses for propane dehydrogenation catalysts. Multiple characterization methods were employed including kinetic studies, XAS, resonance Raman, and IR spectroscopies, and computational methods.  Isolated Co2+, Fe2+, and Ga3+ systems supported on SiO2 were all found to be highly active and selective catalysts.

Extended Abstracts:

See more of: Single Site and Nanoparticle Catalysts (2)
See more of: Catalyst Design and Synthesis
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